Abstract
The previous study of the authors on a phase field method for modelling progressive failure in multi-phase materials is further extended in this study to capture microscopic failure processes in composite laminates. The auxiliary phase field model for the regularization of material interface is re-formulated. In the computational model, a small part of the model is built from microscopic length scale to explicitly consider the microstructure of the material while the other area is built from macroscopic length scale to improve the efficiency. Cohesive elements are employed to link the two mesh parts with different length scales and also to capture the intralaminar failure. The existing ABAQUS subroutine “UEL” has been rewritten for the present study due to the introduction of cohesive elements and a BFGS solver is used to improve the iteration stability. The thickness effect of a thin ply made laminate is considered and the crack suppression effect is investigated.
Introduction
Reinforced composite laminates are now widely used in industrial applications. A deep insight of the failure mechanism at early stages in composite laminates and the left carrying capability is desired. Essentially, composite laminates are multiphase materials. Even for a single lamina, it is composed of fiber, matrix, material interface, voids, defects, etc. From the point of view of a larger length scale, a laminate is made of several laminas by stacking them together with a designed sequence. Although various well designed experiments are available, most of them are conducted and observed from macroscopic length scale, a precise experimental observation of a complete failure process from microscopic length scale is however rather demanding.1–3
In addition to experimental tests, virtual tests that rely on faithful numerical methods may serve as a good alternative. Virtual tests do not require the preparation of specimens and test set up, the job is ran with a computer and thus less costly. The kernel of a virtual test is the numerical method it uses, because it directly decides the modelling accuracy and efficiency. On one hand, we need a full understanding of the global response of laminates from macroscopic length scale. And the relative modelling scheme is more or less well developed. With the increasing demand from engineering, the local failure behavior of the material from microscopic length scale must be taken into consideration. Homogenization schemes used in most of the modelling approaches have prevented it from digging into the mechanical response of the microstructure and thus may bring significant error. So far, a reliable numerical method for the modelling of tensile failure in composite laminate from different length scales is still desired. We thus develop a phase field modelling scheme for this purpose in the present study.
Phase field model for fracture was developed on the basis of the variational principle proposed by Francfort and Marigo. 4 In the variational principle, the total system potential energy functional has further included the energy dissipated for generating new crack surfaces. The dissipated energy is calculated by the critical energy release rate multiplied by the new crack surface area and thus makes the phase field model in consistence with the Griffith’s fracture theory. 5 The phase field value can be solved with given boundary and loading conditions, and crack evolution including, crack nucleation, propagation, branching, etc, can be described by the evolution of the phase field value. 6 In this way, complex failure processes can modelled without any crack tracking strategy. Due to the advantages of the phase field modelling, it attracts great attention. So far, phase field model for fracture has been widely used for ductile fracture problems,7–11 brittle fracture problems,12–21 anisotropic fracture problems,22–27 cohesive fracture problems,28–34 and dynamic fracture problems.35–40 Phase field models are also developed to model material failure process in composite materials.41–45 Phase field is normally computationally expensive for solving the nonlinear equations, a multi-scale modelling scheme in Patil et al. 18 for higher efficiency was thus proposed. Only the area around the crack tip needs to use refined mesh in which the phase field equations are solved, whereas other areas are meshed using coarse meshes. The multi-scale phase field modelling scheme was then further enhanced and extended for more complicated problems i.e., composite materials, heterogeneous materials.46–48 Recently, a few new adaptive mesh refinement strategies were developed for the localizing gradient damage model, and the refinement criterion and data transfer schemes are also studied for higher efficiency. 49
In the previous study, the authors developed a few phase field models for modelling failure process in composites.50–53 Among the contributions, we introduced an auxiliary interface phase field model in Zhang et al. 53 to regularize the interface between inclusion and matrix. Such that the failure process in composite at microscopic length scale involving inclusion debonding and matrix cracking can be modelled effectively. However, the phase field model was developed mostly for modelling damage/failure in a small portion of material in lamina from microscopic length scale, it is inapplicable when failure processes in laminate are investigated. Specially, in a computational model involving multiple length scales, the existing microscopic phase field model needs further enhancement to account for other failure mechanisms such as delamination and the interaction between delamination and matrix cracking.
In this study, the existing modelling scheme is further enhanced to predict microscopic failures in composite laminates. A computational model with multi-grid meshes is introduced in detail, namely, a refined mesh region with randomly distributed fibers from microscopic length scale, and a coarse mesh region with homogenized material properties from macroscopic length scale are used. Cohesive elements are used to link the two parts of the meshes, and also to capture interlaminar failure between layers. The phase field model for the regularization of the material interface between inclusion and matrix is simplified for the fiber reinforced composite and an analytical solution is obtained.
Phase field model of cohesive model based cracks
The basic concept of the phase field model for fracture is depicted in Figure 1, and the fundamental equations are summarized as follows

Explicit and smeared crack models. (a) Explicit model, (b) Smeared model.
In the above equations,
It is noteworthy that for some other common cohesive zone models, the coefficients can also be derived and are available in Wu. 31
An auxiliary phase field for fiber-matrix interface
In the modeling of transverse cracking in composite laminates from microscopic length scale, matrix cracking and fiber-matrix interface debonding are normally considered key failure mechanisms. When modelling such failure processes using the phase field model, CERR is used as an important material property. Although in reality material is continuous over matrix, fiber and the interface, and the material property CERR is thus also continuous, the CERRs of matrix and the interface are normally considered two different material properties. And experimental test procedures were designed to measure the two CERRs. Thus, there is a sudden change of CERR (see Figure 2(b)) without using any regularization scheme. Obviously, the material sudden change (or material heterogeneity) has made the modelling with phase field method challenging. Especially if we want to model failure processes in both the matrix and the interface.

An auxiliary phase field and the distribution of material property (CERR), (a) is the one-dimensional distribution of the auxiliary phase field, (b) is the material property distribution without using the auxiliary phase field regularization, and (c) is the material property distribution using the auxiliary phase field regularization.
In the previous study, 53 the authors have proposed an interface regularization scheme to eliminate the material heterogeneity by introducing an auxiliary phase field termed as the interface phase field (IPF). The previous regularization theory was proposed mostly for concrete or materials in which the shape of the inclusion could be arbitrary. And an image processing scheme by identifying the value of the picture pixels was introduced to distinguish different material phases.
In the present investigation of fiber reinforced composite, the cross section of a fiber is simply a circular. Hence, the auxiliary IPF model can be reformulated, and the identification of the material phases can be conducted through an analytical but simple way. The IPF function
The above one-dimensional (1 D) theory can easily be extended to a two-dimensional (2 D) case, and it is not discussed here for the sake of simplicity.
Generation of the local microscopic computational model
In the previous study,
53
the distribution of
Generation of the global computational model with multi-grid meshes
With the scheme for the generation of microscopic models introduced above, we further generate a multi-grid computational model. Taking the test specimen considered in ‘Validation’ section 8.2 as an example, the pre-processing scheme for other stacking sequences is similar, and details of the pre-processing are depicted in Figure 3. The

The detailed finite element model of the tested specimen.

The IPF distributions in the
In addition to matrix cracking and fiber debonding, delamination between adjacent plies should also be considered when investigating failure processes in composite laminates. According to the existing studies, cohesive element is considered one of the most proper and popular approaches for the modelling of delamination in composite laminates. Cohesive elements are placed along the interface between adjacent plies which essentially is the potential crack path of delamination. Moreover, the numerical predictions by using cohesive elements are very accurate in comparison with experimental observations as reported repeatedly in open literatures. So, we choose to use cohesive elements and insert them into the ply interfaces between the

Interaction between phase field model and cohesive element (“CE” represents cohesive element).
The fiber-matrix interface and the ply interface
In this study, two kinds of material interfaces are involved, i.e., the interface between adjacent plies and the fiber-matrix interface. We use different approaches to capture the interfacial failure processes, e.g., phase field model for the fiber-matrix interface debonding and cohesive element for delamination along the ply interface. Despite the fact that cohesive element is also proven proper and has been widely used for the modelling of fiber debonding, it is still recommended, like in the present modelling strategy, to use phase field model for the modelling of debonding. It is mostly because we consider a more complicated failure mechanism involving fiber debonding, matrix cracking and the interaction between them. Cohesive element might be satisfactory when modelling a single failure mechanism in material interfaces, fiber debonding or delamination, it brings difficulties when combined with other numerical methods for matrix cracking (phase field model in the present study). But in the proposed strategy, the fiber interface is smeared over the surrounding area, and both matrix cracking and fiber debonding are treated with the fracture phase field model. The interaction between fiber debonding and matrix cracking can also be captured automatically with the phase field model, and no more special treatment is required. It is noteworthy that the cohesive elements in between the plies are necessary to link the two mesh parts, the micro-scale dense mesh and the macro-scale coarse mesh. For the case we consider purely a micro-scale model, it is then unnecessary to use cohesive elements.
The present modelling strategy also brings advantages for the generation of computational models. It is known that one of the challenges in modelling heterogeneous material is the generation of computational models because, for example, the arbitrarily distributed fibers and the material property variation among different material phases. Normally, it requires extensive efforts being devoted to analytically build the model topology and identify the material phases. We find that the proposed strategy uses structured mesh with rectangular elements even for the fiber debonding, and the pre-processing is simplified and thus more convenient.
Finite element formulation and the BFGS solver
The formed computational model is solved numerically with finite element method (FEM). The fully coupled nonlinear equation set of the fracture phase field model can be specified by
For this purpose, the stiffness matrix is specified by
For the systems of symmetric stiffness matrix, the inverse of the modified stiffness matrix is explicitly available
In fact, the tangential stiffness matrix
The above stiffness matrix can be guaranteed symmetric and positive-definite in practice. In fact, the modified stiffness matrix
The present theory is implemented into the commercial finite element package ABAQUS through its users’ subroutine (UEL). Both the bulk elements (micro-scale, for the
Verification and validation
Verification
It is considered a square shaped FRP composite sample with 24 randomly placed fibers (volume fraction 42%) as depicted in Figure 6. The width of the sample is

A composite lamina subjected to tensile loading and the distribution of the fibers (unit: micron).
The microstructure and the contours of

Modelling results of the specimen shown in Figure 6, stress-strain curve and failure mode.
Validation
An experiment conducted by Saito et al.,
1
is modelled to further validate the proposed method. In the experiment, a cross-ply composite laminate subjected to a tensile load was tested, and fiber-matrix debonding in the

The experimental set up of Saito’s test. (“N” is the number of the
Due to the limit of computational costs, only a part of the specimen with a length of 0.12 mm is modelled in this study, see the right sub-figure of Figure 8. A parametric study with 0.15 mm, 0.18 mm, and 0.20 mm has been conducted, and the results suggest that 0.12 mm is adequate because modellings with other lengths give converged results.
The crack patterns at different loading stages are shown in Figure 9, in which the dark curves represent intralaminar failures (matrix-fiber debonding are matrix cracking) and the pink line segments are interlaminar failures (delamination). The intralaminar failure patterns are generated automatically using a “Tecplot” software with the calculation results. The intralaminar failure patterns are drawn artificially using a “Photoshop” software onto the former failure pattern based on the calculation results. The whole failure processing is divided into five stages as shown in Figure 9, i.e., the tensile strain reaches 0.5%, 0.8%, 1.0%, 1.5%, 2.0%. We term the five stages “stage I, II, III, VI and V” for simplicity. The three specimens mainly undergo an elastic stage from the start to “stage I” since not a clear damage pattern is observed. Intralaminar failure is found in “stage II” for all the specimens. Fiber-matrix debonding takes place first and kinks into the matrix, the cracks then merge with each other. Once reaching the ply interface, the previously formed intralaminar crack could then trigger a delamination. The first delamination triggered by the matrix crack is observed in the specimen with 4 layers of

Numerical prediction of the failure process (black curves represent intralaminar failure while pink lines represent interlaminar failure).
The variation of crack density (which is defined by the total crack length in the thickness direction divided by the thickness of the

Crack density vs. tensile strain, present prediction and the experimental results. 2
Numerical predictions of crack pattern when crack density reaches 1.0 are depicted in Figure 11, in which the experimental observations are provided. In comparison with thick-ply composites, matrix crack is also shorter in thin-ply composites. It is known that stress intensity factors at the crack tips of longer cracks are normally larger and thus easier to trigger another crack (delamination in this case). And this explains why the delamination in Figure 9 for

Crack paths obtained from the experimental test 2 and the present modelling.
Conclusion
As an extension of the previous study, the auxiliary interface phase field model is in fact a special case of the general model for the inclusion with arbitrary shape. The auxiliary interface phase field model is thus analytically derived and explicitly specified. Composite lamina with complex microstructure shapes can be modelled on a regular mesh with rectangular elements with the proposed model. The introduction of cohesive elements in the computational model has made it possible to capture the interlaminar failure. The proposed phase field modelling scheme is effective in capturing a complicated failure process with multiple failure mechanisms in composite laminates. In addition to the findings reported in Saito et al., 2 the present numerical results suggest that the suppression of delamination could be another crack suppression mechanism of thin-ply composites. The crack suppression capability of a laminate is found to have a direct correlation with its capability in limiting the length of matrix cracks.
Footnotes
Acknowledgement
Professor Hiroshi Saito is sincerely appreciated for providing material properties and experimental data.
Declaration of Conflicting Interests
The author(s) declared no potential conflicts of interest with respect to the research, authorship, and/or publication of this article.
Funding
The author(s) disclosed receipt of the following financial support for the research, authorship, and/or publication of this article: This work was supported by the National Natural Science Foundation of China (No. 11872143) and the National Key Research and Development Program of China [No.2016YFB0200702].
