Abstract
Physical evaporation of SiO and SiO2 under ultra-high vacuum conditions was monitored in situ with infrared spectroscopy at frequencies between 450 cm−1 and 5000 cm−1. The measured vibrational spectra of the condensed films are identical in both cases, for SiO and SiO2 evaporation, and can be described with four Brendel oscillators located at 380 cm−1, 713 cm−1, 982 cm−1, and 1101 cm−1, corresponding to typical vibration modes in SiO.
References
1.
van Boekel
R.
Min
M.
Leinert
C.
Waters
L. B. F. M.
Richichi
A.
Chesneau
O.
Dominik
C.
Jaffe
W.
Dutrey
A.
Graser
U.
, Nature 432 , 479 (2004 ).
2.
Gail
H. P.
and
Sedlmayr
E
, Astron. Astrophys. 347 , 594 (1999 ).
3.
Gail
H. P.
and
Sedlmayr
E
, Astron. Astrophys. 166 , 225 (1986 ).
4.
Gail
H. P.
, Astron. Astrophys. 413 , 571 (2004 ).
5.
Nesbit
L. A.
, Appl. Phys. Lett. 46 , 38 (1985 ).
6.
Hohl
A.
Wieder
T.
van Aken
P. A.
Weirich
T. E.
Denninger
G.
Vidal
M.
Oswald
S.
Deneke
C.
Mayer
J.
and
Fuess
H
, J. Non-Cryst. Solids 320 , 255 (2003 ).
7.
Friede
B.
and
Jansen
M
, J. Non-Cryst. Solids 204 , 202 (1996 ).
8.
Nakamura
M.
Mochizuki
Y.
Usami
K.
Itoh
Y.
and
Nozaki
T
, Solid State Commun. 50 , 1079 (1984 ).
9.
Howson
R.
, Thin Solid Films 9 , 109 (1972 ).
10.
Hass
G.
, J. Am. Ceram. Soc. 33 , 353 (1950 ).
11.
Philipp
H.
, J. Phys. Chem. Solids 32 , 1935 (1971 ).
12.
Hass
G.
and
Salzberg
C. D
, J. Opt. Soc. Am. 44 , 181 (1954 ).
13.
Tazawa
M.
Kakiuchida
H.
Xu
G.
Jin
P.
and
Arwin
H
, J. Electroceram. 16 , 511 (2006 ).
14.
Klevenz
M.
Wetzel
S.
Trieloff
M.
Gail
H. P.
and
Pucci
A
, Phys. Stat. Sol. B, paper submitted (2009 ).
15.
Schick
H. L.
, Chem. Rev. 60 , 331 (1960 ).
16.
Ferguson
F. T.
and
Nuth
J. A
, J. Chem. Eng. Data 53 , 2824 (2008 ).
17.
Brewer
L.
and
Mastick
D. F
, J. Chem. Phys. 19 , 834 (1951 ).
18.
Berreman
D. W.
, Phys. Rev. 130 , 2193 (1963 ).
19.
Lehmann
A.
, Phys. Stat. Sol. B 148 , 401 (1988 ).
20.
Teschner
U.
and
Hübner
K
, Phys. Stat. Sol. B 159 , 917 (1990 ).
21.
Galeener
F. L.
and
Lucovsky
G
, Phys. Rev. Lett. 37 , 1474 (1976 ).
22.
Fuchs
R.
and
Kliewer
K. L
, Phys. Rev. 140 , 2076 (1965 ).
23.
Ibach
H.
and
Mills
D
, Electron Energy Loss Spectroscopy and Surface Vibrations (Academic Press , New York , 1982 ).
24.
Lehmann
A.
, Phys. Stat. Sol. B 166 , 525 (1991 ).
25.
Lehmann
A.
and
Mutschke
H
, Phys. Stat. Sol. A 125 , 363 (1991 ).
26.
Brendel
R.
and
Bormann
D
, J. Appl. Phys. 71 , 1 (1992 ).
27.
Lehmann
A.
Schumann
L.
and
Hübner
K
, Phys. Stat. Sol. B 121 , 505 (1984 ).
28.
Lehmann
A.
, Thesis , Friedrich Schiller University of Jena (1993 ).
29.
Kirk
C. T.
, Phys. Rev. B 38 , 1255 (1988 ).
30.
Chabal
Y. J.
Raghavachari
K.
Zhang
X.
and
Garfunkel
E
, Phys. Rev. B 66 , 161315 (2002 ).
31.
Dorn
R.
Lüth
H.
and
Ibach
H
, Surf. Sci. 42 , 583 (1974 ).
32.
Violanda
M. L.
and
Rudolph
H
, Surf. Sci. 603 , 901 (2009 ).
33.
Lehmann
A.
, Thin Solid Films 230 , 55 (1993 ).
34.
Persson
B. N. J.
and
Ryberg
R
, Phys. Rev. B 24 , 6954 (1981 ).
35.
Theiss
M.
, Scout–software package for optical spectroscopy .
36.
Hjortsberg
A.
and
Granqvist
C. G
, Appl. Opt. 19 , 1694 (1980 ).
37.
Ishikawa
K.
Suzuki
K.
and
Okamura
S
, J. Appl. Phys. 88 , 7150 (2000 ).
38.
Grosse
P.
Harbecke
B.
Heinz
B.
and
Meyer
R
, Appl. Phys. A 39 , 257 (1986 ).
39.
Naiman
M. L.
Kirk
C. T.
Emerson
B. L.
Taitel
J. B.
and
Senturia
S. D
, J. Appl. Phys. 58 , 779 (1985 ).
40.
Palik
E.
, Handbook of Optical Constants of Solids II (Academic Press , New York , 1991 ).
41.
Montalenti
F.
and
Voter
A. F
, Phys. Rev. B 64 , 081401 (2001 ).